Development of Smart Materials for Self-Healing Structural Applications

Authors

  • Dedi Gunawan Saputra Universitas Negeri Makassar
  • Dewi Suryaningsih Saputri STIE IEU Surabaya

DOI:

https://doi.org/10.63891/j-mart.v1i3.33

Keywords:

self-healing, smart materials, durability, cementitious, composites

Abstract

Self-healing materials are increasingly explored for structural applications because they can autonomously repair damage, reduce maintenance needs, and extend service life. Structural components frequently experience microcracking caused by cyclic loading, shrinkage, thermal variation, and environmental exposure. If not addressed, these cracks may grow and accelerate deterioration, leading to higher lifecycle costs and reduced reliability. This study aimed to systematically review and synthesize recent research on smart self-healing materials for structural applications by mapping material classes, healing mechanisms, and performance evaluation practices reported in the literature. A systematic review method was applied using structured database searches, duplicate removal, title and abstract screening, and full-text eligibility assessment based on predefined inclusion and exclusion criteria. Eligible peer-reviewed studies were required to report measurable healing outcomes. Data were extracted using a standardized form and organized by material type, healing approach, test methods, and outcome metrics. The results showed that cementitious materials dominated the included literature, followed by polymer-based systems and composite materials. Microcapsule-based healing was the most frequently investigated mechanism, while intrinsic healing and biologically driven healing approaches were also widely reported. Across studies, crack closure and mechanical strength recovery were the most commonly used indicators of healing effectiveness, whereas permeability reduction and durability-related indicators were reported less consistently. Overall, the evidence indicates strong research momentum in demonstrating healing functionality under controlled conditions, but also highlights variability in testing methods and outcome definitions across studies. This review provides a structured evidence map to support material selection, improve comparability of future studies, and guide the development of standardized evaluation approaches for practical structural deployment.

References

Bekas, D. G., Tsirka, K., Baltzis, D., & Paipetis, A. S. (2016). Self-healing materials: A review of advances in materials, evaluation, characterization and monitoring techniques. Composites Part B: Engineering, 87, 92–119. https://doi.org/10.1016/j.compositesb.2015.09.057

Blaiszik, B. J., Kramer, S. L. B., Olugebefola, S. C., Moore, J. S., Sottos, N. R., & White, S. R. (2010). Self-healing polymers and composites. Annual Review of Materials Research, 40, 179–211. https://doi.org/10.1146/annurev-matsci-070909-104532

de Rooij, M., van Tittelboom, K., De Belie, N., & Schlangen, E. (2013). Self-healing phenomena in cement-based materials. Springer. https://doi.org/10.1007/978-94-007-6624-2

Guimard, N. K., Oehlenschlaeger, K. K., Zhou, J., Hilf, S., Schmidt, F. G., & Barner-Kowollik, C. (2012). Current trends in the field of self-healing materials. Macromolecular Chemistry and Physics, 213(2), 131–143. https://doi.org/10.1002/macp.201100442

Hager, M. D., Greil, P., Leyens, C., van der Zwaag, S., & Schubert, U. S. (2010). Self-healing materials. Advanced Materials, 22(47), 5424–5430. https://doi.org/10.1002/adma.201003036

Hansen, C. J., Wu, W., Toohey, K. S., Sottos, N. R., White, S. R., & Lewis, J. A. (2009). Self-healing materials with interpenetrating microvascular networks. Advanced Materials, 21(41), 4143–4147. https://doi.org/10.1002/adma.200900588

Jonkers, H. M., Thijssen, A., Muyzer, G., Copuroglu, O., & Schlangen, E. (2010). Application of bacteria as self-healing agent for the development of sustainable concrete. Ecological Engineering, 36(2), 230–235. https://doi.org/10.1016/j.ecoleng.2008.12.036

Liao, C.-Y., Zhang, L., Hu, S.-Y., Xia, S.-J., & Li, D.-M. (2024). Recent advances of self-healing materials for civil engineering: Models and simulations. Buildings, 14(4), 961. https://doi.org/10.3390/buildings14040961

Luo, M., Qian, C.-X., & Li, R.-Y. (2015). Factors affecting crack repairing capacity of bacteria-based self-healing concrete. Construction and Building Materials, 87, 1–7. https://doi.org/10.1016/j.conbuildmat.2015.03.117

Page, M. J., McKenzie, J. E., Bossuyt, P. M., Boutron, I., Hoffmann, T. C., Mulrow, C. D., Shamseer, L., Tetzlaff, J. M., Akl, E. A., Brennan, S. E., Chou, R., Glanville, J., Grimshaw, J. M., Hróbjartsson, A., Lalu, M. M., Li, T., Loder, E. W., Mayo-Wilson, E., McDonald, S., … Moher, D. (2021). The PRISMA 2020 statement: An updated guideline for reporting systematic reviews. BMJ, 372, n71. https://doi.org/10.1136/bmj.n71

Toohey, K. S., Sottos, N. R., Lewis, J. A., Moore, J. S., & White, S. R. (2007). Self-healing materials with microvascular networks. Nature Materials, 6(8), 581–585. https://doi.org/10.1038/nmat1934

Van Tittelboom, K., & De Belie, N. (2013). Self-healing in cementitious materials A review. Materials, 6(6), 2182–2217. https://doi.org/10.3390/ma6062182

Wang, S., & Urban, M. W. (2020). Self-healing polymers. Nature Reviews Materials, 5, 562–583. https://doi.org/10.1038/s41578-020-0202-4

White, S. R., Sottos, N. R., Geubelle, P. H., Moore, J. S., Kessler, M. R., Sriram, S. R., Brown, E. N., & Viswanathan, S. (2001). Autonomic healing of polymer composites. Nature, 409(6822), 794–797. https://doi.org/10.1038/35057232

Wool, R. P. (2008). Self-healing materials: A review. Soft Matter, 4, 400–418. https://doi.org/10.1039/B711716G

Downloads

Published

2025-07-13